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Benedict Cumberbatch
Vincent Van Gogh

Jamie Parker
Theo Van Gogh

Aidan McArdle
Paul Gauguin

Christopher Good
Theodorus Van Gogh

Rowena Cooper
Anna Van Gogh

Daniel Weyman
Anthon Van Rappard

Ferdinand Kingsley
Albert Aurier

David Baron
Bernard Soule

Stephanie Jacob
Marguerite Crevlin

Katherine Kanter
Jeanne Coulomb

Richard Trinder
Dr. Peyron

Jim Creighton
Felix Ray

Alan Yentob
Self - Narrator

Vincent van Gogh
Self (archive footage)